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南京航空航天大学 核科学与工程系,江苏 南京,211106
纸质出版日期:2019-3-5,
网络出版日期:2018-6-13,
收稿日期:2018-5-4,
修回日期:2018-6-30,
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陈旺, 汤晓斌, 刘云鹏等. 基于全无机钙钛矿量子点辐致荧光效应的同位素电池研究[J]. 发光学报, 2019,40(3): 326-333
CHEN Wang, TANG Xiao-bin, LIU Yun-peng etc. Study on All-inorganic Perovskite Quantum Dot Radioluminescence Isotope Batteries[J]. Chinese Journal of Luminescence, 2019,40(3): 326-333
陈旺, 汤晓斌, 刘云鹏等. 基于全无机钙钛矿量子点辐致荧光效应的同位素电池研究[J]. 发光学报, 2019,40(3): 326-333 DOI: 10.3788/fgxb20194003.0326.
CHEN Wang, TANG Xiao-bin, LIU Yun-peng etc. Study on All-inorganic Perovskite Quantum Dot Radioluminescence Isotope Batteries[J]. Chinese Journal of Luminescence, 2019,40(3): 326-333 DOI: 10.3788/fgxb20194003.0326.
辐致光伏效应同位素电池因其具有小型化、长寿命等特点,已被广泛研究。研究工作主要致力于提升同位素电池的输出性能。本研究选取全无机钙钛矿量子点作为荧光材料,利用其发射光可调的特性以匹配不同的后端光伏器件,调控优化后同位素电池的最大输出功率显著提升,可提高2.51~3.97倍。基于上述研究结果讨论了优化后端器件的适配性对于核探测和核医学成像等领域的应用价值和参考意义。
Radioluminescence isotope batteries have been extensively studied for their small size and long lifetime. The research work on isotope batteries is mainly aimed at improving the output performance. In this study
all-inorganic perovskite quantum dots were selected as fluorescent materials to match different photovoltaic devices with their tunable emission spectra. The maximum output power of the isotope battery is significantly increased after the spectral regulation
and can be increased by 2.51-3.97 times. At the same time
the application value and reference significance of spectral regulation in nuclear detection and nuclear medicine imaging are discussed.
全无机钙钛矿量子点辐致光伏效应同位素电池光谱调控
all-inorganic perovskite quantum dotsradioluminescence isotope batteryspectral regulation
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HONG L,TANG X B,XU Z H,et al.. Radioluminescent nuclear batteries with different phosphor layers[J]. Nucl. Instrum. Methods Phys. Res. Sect. B:Beam Interact. Mater. At., 2014,338:112-118.
TANG X B,LIANG H,XU Z H,et al.. Temperature effect of a radioluminescent nuclear battery based on147Pm/ZnS:Cu/GaAs[J]. Appl. Radiat. Isot., 2015,97:118-124.
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余彬海,卢汉光,饶龙石,等. 微通道反应器合成高质量的无机钙钛矿量子点及其LED应用[J]. 发光学报, 2018,39(4):440-448. YU B H,LU H G,RAO L S,et al.. Synthesis of high quality inorganic perovskite quantum dots via microchannel reactor and their application in LED[J]. Chin. J. Lumin., 2018,39(4):440-448. (in Chinese)
王俊,禹豪,张继华,等. 采用MoO3阳极缓冲层的钙钛矿太阳能电池研究[J]. 发光学报, 2018,39(3):322-328. WANG J,YU H,ZHANG J H,et al.. Study on perovskite solar cells with MoO3 anode buffer layer[J]. Chin. J. Lumin., 2018,39(3):322-328. (in Chinese)
PROTESESCU L,YAKUNIN S,BODNARCHUK M I,et al.. Nanocrystals of cesium lead halide perovskites (CsPbX3,X=Cl,Br,and I):novel optoelectronic materials showing bright emission with wide color gamut[J]. Nano Lett., 2015,15(6):3692-3696.
NIKOLOPOULOS D,VALAIS I,MICHAIL C,et al.. Radioluminescence properties of the CdSe/ZnS quantum dot nanocrystals with analysis of long-memory trends[J]. Radiat. Meas., 2016,92:19-31.
VALAIS I, NIKOLOPOULOS D, KALIVAS N, et al.. A systematic study of the performance of the CsI:Tl single-crystal scintillator under X-ray excitation[J]. Nucl. Instrum. Methods Phys. Res., 2007,571(1-2):343-345.
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