新兴零维金属卤化物的光致发光与应用研究进展

苏彬彬; 夏志国

doi:10.37188/CJL.20210088

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新兴零维金属卤化物的光致发光与应用研究进展

封面文章 | 更新时间：2021-06-18

- 新兴零维金属卤化物的光致发光与应用研究进展
  增强出版
- Research Progresses of Photoluminescence and Application for Emerging Zero-dimensional Metal Halides Luminescence Materials
- 发光学报 2021年42卷第6期页码：733-754
- 作者机构：
  
  1.华南理工大学材料科学与工程学院发光材料与器件国家重点实验室，广东省光纤激光材料与应用技术重点实验室, 广东广州　 510640
  2.华南理工大学物理与光电学院, 广东广州　 510640
- 作者简介：
  
  [ "苏彬彬(1991-)，男，陕西延安人，博士研究生，2018年于西安建筑科技大学获得硕士学位，主要从事新型零维金属卤化物发光材料的研究。E-mail: 906565162@qq.com" ]
  [ "夏志国(1979-)，男，湖北黄陂人，博士，教授，2008年于清华大学获得博士学位，主要从事稀土掺杂固体发光材料和新型金属卤化物发光材料的研究。E-mail:xiazg@scut.edu.cn" ]
- 基金信息：
  
  国家自然科学基金(51961145101;51972118);广州市科技计划(202007020005);广东省珠江人才计划本地创新团队项目(2017BT01X137)
- DOI：10.37188/CJL.20210088
  中图分类号：
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苏彬彬, 夏志国. 新兴零维金属卤化物的光致发光与应用研究进展[J]. 发光学报, 2021,42(6):733-754.

Bin-bin SU, Zhi-guo XIA. Research Progresses of Photoluminescence and Application for Emerging Zero-dimensional Metal Halides Luminescence Materials[J]. Chinese Journal of Luminescence, 2021,42(6):733-754.
苏彬彬, 夏志国. 新兴零维金属卤化物的光致发光与应用研究进展[J]. 发光学报, 2021,42(6):733-754. DOI： 10.37188/CJL.20210088.

Bin-bin SU, Zhi-guo XIA. Research Progresses of Photoluminescence and Application for Emerging Zero-dimensional Metal Halides Luminescence Materials[J]. Chinese Journal of Luminescence, 2021,42(6):733-754. DOI： 10.37188/CJL.20210088.

摘要

零维(0D)金属卤化物是一类新兴的发光材料体系，它们具有独特的“主-客”体结构，即独立的阴离子金属卤化物多面体客体规则有序地分布在有机阳离子或碱金属阳离子形成的主体框架中。这种具有相对较“软”晶格的0D金属卤化物材料的发光主要源于自陷激子(Self-trapped excitons,STEs)复合，其通常呈现出宽带发射，且具有大的斯托克斯位移。通过筛选不同的及多样化构型的金属卤化物多面体，将其与合适的有机阳离子或者Cs,+,等组合，可形成多种新型结构的0D金属卤化物，并实现丰富的STEs发光特性，其可调节的荧光发射不仅可以覆盖整个可见光区，还可实现单相白光或近红外发光，成为光致发光材料研究领域的一个热点和重点。基于此，本文结合本课题组在该领域的研究工作基础，首先讨论了0D金属卤化物的光致发光机理;其次，介绍了具有不同多面体构型的0D金属卤化物材料的发光特性及应用;最后，总结了0D金属卤化物目前亟待解决的关键科学问题，并对0D金属卤化物的未来发展方向进行了展望。

Abstract

Zero-dimensional(0D) metal halides belong to a new kind of luminescent materials, and they have the unique "host-guest" structure, in which the isolated anionic metal halide polyhedrons are regularly distributed in the main body of organic cations or alkali metal ions. Generally, 0D metal halides with relatively "soft" lattice usually present broad band emission with large Stokes shift, and their luminescence mechanism is mainly derived from self-trapped excitons(STEs) recombination. By screening different metal halide polyhedrons with diversified configurations, one can combine them with appropriate organic cations or alkali metal ions to form new 0D metal halides with different structure types. The obtained 0D metal halides show rich STEs luminescence properties, and their tunable fluorescence emission can be available to cover the entire visible light region. Moreover, it can also realize single-phase white light emission or near infrared emission, making them become a hot spot in the field of photoluminescence materials. Based on our work and others in this field, the photoluminescence mechanisms of 0D metal halides are firstly discussed in this review. Secondly, the luminescence properties and applications of 0D metal halide materials with different polyhedron configurations are introduced. Finally, the key scientific problems of 0D metal halides during the development are summarized, and the future research direction is briefly proposed.

关键词

金属卤化物光致发光LED应用

Keywords

metal halidesphotoluminescenceLED application

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