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1. 天津理工大学 理学院 天津,300384
2. 天津理工大学 显示技术与光电器件教育部重点实验室, 天津 300384
纸质出版日期:2017-11-5,
网络出版日期:2017-9-11,
收稿日期:2017-4-21,
修回日期:2017-5-19,
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常鑫鑫, 沈礼, 杨玉娜等. 铕原子4f<sup>7</sup>6p<sub>3/2</sub><em>n</em>d自电离态的光谱[J]. 发光学报, 2017,38(11): 1461-1468
CHANG Xin-xin, SHEN Li, YANG Yu-na etc. Spectra of Eu 4f<sup>7</sup>6p<sub>3/2</sub><em>n</em>d Autoionizing States[J]. Chinese Journal of Luminescence, 2017,38(11): 1461-1468
常鑫鑫, 沈礼, 杨玉娜等. 铕原子4f<sup>7</sup>6p<sub>3/2</sub><em>n</em>d自电离态的光谱[J]. 发光学报, 2017,38(11): 1461-1468 DOI: 10.3788/fgxb20173811.1461.
CHANG Xin-xin, SHEN Li, YANG Yu-na etc. Spectra of Eu 4f<sup>7</sup>6p<sub>3/2</sub><em>n</em>d Autoionizing States[J]. Chinese Journal of Luminescence, 2017,38(11): 1461-1468 DOI: 10.3788/fgxb20173811.1461.
利用三步三色孤立实激发技术(ICE),系统地研究了铕原子4f
7
6p
3/2
n
d自电离态的光谱,同时首次研究了激光偏振对复杂原子的光谱的影响。为了研究铕原子4f
7
6p
3/2
n
d自电离态的光谱,首先设计并采用了不同的激发路径,分别将原子布居到同一高激发能域并探测它们在该能域的自电离光谱。通过比较这些光谱的异同并结合上述激发路径所对应的跃迁选择定则,便可唯一地确定这些高激发态的总角动量。为了研究激光偏振对铕原子的影响,设计并使用了两种偏振组合:三步激光都是垂直(),三步激光都是平行()(激光偏振方向相对于探测器垂直或平行)。为了得到有偏振影响的光谱,分别使3部激光器处于同一偏振,依次对铕原子进行激发,激发路径与终态同上。通过对同一路径不同偏振下的光谱的比较,发现仅能确定极少数的高激发态的总角动量,同时在光谱中一些峰独立于另一偏振光谱存在。
Experimental spectra of the Eu 4f
7
6p
3/2
n
d(
n
=6
7) autoionizing states were investigated by using the three-step isolated-core excitation technique
while the impact of laser polarization on the spectra was studied for the first time. A detailed interpretation to the complex spectra of the 4f
7
6p
3/2
n
d (
n
=6
7) autoionizing states is fulfilled by reproducing their line shapes with a multi-peaked fitting process. The spectroscopic information of the autoionizing states
like the total angular momentum (
J
is deduced by comparing their corresponding spectra obtained under different excitation paths.
铕原子自电离光谱激光偏振选择定则
Eu atomspectrum of autoionizing statelaser polarizationselection rules
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