GaAsN/GaAs量子阱在1 MeV电子束辐照下的退化规律

雷琪琪; 郭旗; 艾尔肯·阿不都瓦衣提; 玛丽娅·黑尼; 李豫东; 王保顺; 王涛; 莫镜辉; 庄玉; 陈加伟

doi:10.3788/fgxb20204105.0603

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GaAsN/GaAs量子阱在1 MeV电子束辐照下的退化规律

发光学应用及交叉前沿 | 更新时间：2020-09-21

- GaAsN/GaAs量子阱在1 MeV电子束辐照下的退化规律
- Degradation of GaAsN/GaAs Quantum Well Under 1 MeV Electron Beam Irradiation
- 发光学报 2020年41卷第5期页码：603-609
- 作者机构：
  
  1.中国科学院新疆理化技术研究所, 中国科学院特殊环境功能材料与器件重点实验室, 新疆电子信息材料与器件重点实验室, 新疆乌鲁木齐 830011
  2.中国科学院大学, 北京 100049
  3.云南师范大学能源与环境科学学院, 云南昆明 650500
  4.新疆大学物理科学与技术学院, 新疆乌鲁木齐 830046
- 作者简介：
  
  [ "雷琪琪(1994-), 男, 甘肃陇西人, 硕士研究生, 2017年于新疆大学获得学士学位, 主要从事太阳电池和稀氮材料(Ga (In) AsN)辐射效应的研究。E-mail:1243642152@qq.com" ]
  [ "郭旗(1964-), 男, 新疆乌鲁木齐人, 学士, 研究员, 博士研究生导师, 1986年于北京理工大学获得学士学位, 主要从事光电材料与器件空间辐射效应方面的研究。E-mail:guoqi@ms.xjb.ac.cn" ]
- 基金信息：
  
  国家自然科学基金(61534008);中国科学院新疆理化技术研究所所长基金(Y55B171101);中科院西部之光(2017-XBQNXZ-B-004);电子元器件可靠性物理及其应用技术重点实验室开放基金(ZHD201705)
- DOI：10.3788/fgxb20204105.0603
  中图分类号：
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雷琪琪, 郭旗, 艾尔肯·阿不都瓦衣提, 等. GaAsN/GaAs量子阱在1 MeV电子束辐照下的退化规律[J]. 发光学报, 2020,41(5):603-609.

Qi-qi LEI, Qi GUO, ABUDUWAYITI Aierken, et al. Degradation of GaAsN/GaAs Quantum Well Under 1 MeV Electron Beam Irradiation[J]. Chinese Journal of Luminescence, 2020,41(5):603-609.
雷琪琪, 郭旗, 艾尔肯·阿不都瓦衣提, 等. GaAsN/GaAs量子阱在1 MeV电子束辐照下的退化规律[J]. 发光学报, 2020,41(5):603-609. DOI： 10.3788/fgxb20204105.0603.

Qi-qi LEI, Qi GUO, ABUDUWAYITI Aierken, et al. Degradation of GaAsN/GaAs Quantum Well Under 1 MeV Electron Beam Irradiation[J]. Chinese Journal of Luminescence, 2020,41(5):603-609. DOI： 10.3788/fgxb20204105.0603.

摘要

为研究GaAsN/GaAs量子阱在电子束辐照下的退化规律与机制，对GaAsN/GaAs量子阱进行了不同注量（1×10,15,，1×10,16, e/cm,2,）1 MeV电子束辐照和辐照后不同温度退火（650，750，850 ℃）试验，并结合Mulassis仿真和GaAs能带模型图对其分析讨论。结果表明，随着电子注量的增加，GaAsN/GaAs量子阱光学性能急剧降低，注量为1×10,15, e/cm,2,和1×10,16, e/cm,2,的电子束辐照后，GaAsN/GaAs量子阱PL强度分别衰减为初始值的85%和29%。GaAsN/GaAs量子阱电子辐照后650 ℃退火5 min，样品PL强度恢复到初始值，材料带隙没有发生变化。GaAsN/GaAs量子阱辐照后750 ℃和850 ℃各退火5 min后，样品PL强度随退火温度的升高不断减小，同时N原子外扩散使得样品带隙发生约4 nm蓝移。退火温度升高没有造成带隙更大的蓝移，这是由于进一步的温度升高产生了新的N—As间隙缺陷，抑制了N原子外扩散，同时导致GaAsN/GaAs量子阱光学性能退化。

Abstract

The radiation effects of MBE grown GaAsN/GaAs quantum well irradiated by 1 MeV electron with different dose (1×10,15, 1×10,16, e/cm,2,) and post thermal annealing (650, 750, 850℃) have been studied.The degradation mechanism and annealing effects were discussed by Mulassis simulation and GaAs energy bandgap model. The results show that the GaAsN/GaAs quantum well PL intensity significantly decreased with the increase of electron does. The PL intensity of the GaAsN GaAs quantum well decayed to 85% and 29% of the initial value after electron irradiation with doses of 1×10,15, e/cm,2, and 1×10,16, e/cm,2, respectively. The PL intensity of GaAsN/GaAs quantum well returned to original value after annealing at 650℃ for 5 min, and the bandgap of the material remained unchanged. The PL intensity of GaAsN/GaAs samples decreased as the annealing temperature increased after annealed at 750℃ and 850℃ for 5 min, and the bandgap blue shifted about 4 nm due to the diffusion of N atoms from GaAsN quantum well to GaAs barrier layer. The increase of annealing temperature did not cause additional blue shifts of the band gap. This was due to the further increase in temperature, which caused new N-As defects, suppressed N-atom diffusion, and degraded the optical properties of GaAsN/GaAs quantum well.

关键词

稀氮光致发光电子辐照GaAsN退火

Keywords

dilute nitridephotoluminescenceelectron irradiationGaAsNannealed

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