浏览全部资源
扫码关注微信
发光学及应用国家重点实验室 中国科学院长春光学精密机械与物理研究所,吉林 长春,130033
收稿日期:2014-06-03,
修回日期:2014-07-16,
纸质出版日期:2014-09-03
移动端阅览
曲松楠, 刘星元, 申德振. 氮掺杂发光碳纳米点的研究探索[J]. 发光学报, 2014,35(9): 1019-1026
QU Song-nan, LIU Xing-yuan, SHEN De-zhen. Studies on Nitrogen-dopped Carbon Nanodots[J]. Chinese Journal of Luminescence, 2014,35(9): 1019-1026
曲松楠, 刘星元, 申德振. 氮掺杂发光碳纳米点的研究探索[J]. 发光学报, 2014,35(9): 1019-1026 DOI: 10.3788/fgxb20143509.1019.
QU Song-nan, LIU Xing-yuan, SHEN De-zhen. Studies on Nitrogen-dopped Carbon Nanodots[J]. Chinese Journal of Luminescence, 2014,35(9): 1019-1026 DOI: 10.3788/fgxb20143509.1019.
采用微波法制备了氮掺杂碳纳米点。通过调控碳纳米点中氮元素的掺杂含量和表面的化学环境,实现了对碳纳米点发光特性的调控。在此基础上,可实现完全基于氮掺杂碳纳米点的荧光墨水、比率型荧光探针及光泵浦激光。研究目的在于探索氮掺杂碳纳米点的发光机理,揭示影响碳纳米点荧光量子效率的因素及其在生物成像、传感、防伪、信息存储、激光等领域的应用。
Nitrogen-dopped carbon nanodots are emerging stars in carbon-based nanomaterials. Herein
we introduce our works on nitrogen-dopped nanodots
which were prepared through one-step microwave synthesis route. Our works demonstrated that the optical properties of the carbon nanodots can be modulated by nitrogen dopping concentrations and surface chemical environments
and realize carbon-nanodot-based fluorescent inks
ratiometric fluorescent nanosensor and optical pumped laser. Our studies aim at exploiting the luminescent mechanism of the nitrogen-dopped carbon nanodots
revealing the influencing factors on their luminescent quantum yields and their applications in bioimaging
sensing security
information storage
lasers and so on.
Xu X, Ray R, Gu Y, et al. Electrophoretic analysis and purification of fluorescent single-walled carbon nanotube fragments [J]. J. Am. Chem. Soc., 2004, 126(40):12736-12737.
Sun Y P, Zhou B, Lin Y, et al. Quantum-sized carbon dots for bright and colorful photoluminescence [J]. J. Am. Chem. Soc., 2006, 128(24):7756-7757.
Baker S N, Baker G A. Luminescent carbon nanodots: Emergent nanolights [J]. Angew. Chem. Int. Ed., 2010, 49(38): 6726-6744.
Xie Z, Wang F, Liu C. Organic-inorganic hybrid functional carbon dot gel glasses [J]. Adv. Mater., 2012, 24(13): 1716-1721.
Zhu S, Meng Q, Wang L, et al. Highly photoluminescent carbon dots for multicolor patterning, sensors, and bioimaging [J]. Angew. Chem. Int. Ed., 2013, 52(14):3953-3957.
Qu S N, Wang X Y, Lu Q P, et al. New type of biocompatible fluorescent ink based on water-soluble luminescent carbon nanodots [J]. Angew. Chem. Int. Ed., 2012, 51(49):12215-12218.
Shi W, Li X H, Ma H M. A tunable ratiometric pH sensor based on carbon nanodots for the quantitative measurement of the intracellular pH of whole cells [J]. Angew. Chem. Int. Ed., 2012, 51(26):6432-6435.
Zhu A, Qu Q, Shao X, et al. Carbon-dot-based dual-emission nanohybrid produces a ratiometric fluorescent sensor for in vivo imaging of cellular copper Ions [J]. Angew. Chem. Int. Ed., 2012, 51(29):7185-7189.
Qu S N, Chen H, Zheng X M, et al. Ratiometric fluorescent nanosensor based on water soluble carbon nanodots with multiple sensing capacities [J]. Nanoscale, 2013, 5(12):5514-5518.
Zhang W F, Zhu H, Yu S F, et al. Observation of lasing emission from carbon nanodots in organic solvents [J]. Adv. Mater., 2012, 24(17):2263-2267.
Liu F, Jang M, Ha H D, et al. Facile synthetic method for pristine graphene quantum dots and graphene oxide quantum dots: Origin of blue and green luminescence [J]. Adv. Mater., 2013, 25(27):3657-3662.
Qu S N, Liu X Y, Guo X Y, et al. Amplified spontaneous green emission and lasing emission from carbon nanoparticles [J]. Adv. Funct. Mater., 2014, 24(18):2689-2695.
Qu S N, Shen D Z, Liu X Y, et al. Highly luminescent carbon-nanoparticle-based materials: Factors influencing photoluminescence quantum yield [J]. Part. Part. Syst. Charact., 2014, DOI: 10.1002/ppsc.201400055.
0
浏览量
116
下载量
6
CSCD
关联资源
相关文章
相关作者
相关机构