Construction of Quantum Dot-modified <italic style="font-style: italic">Ln</italic>-ZIF Hybrid Materials and Fluorescence Detection of Tannic Acid

FANG Zhou; JIA Dongsheng; LI Tianming; LI Ying; ZHANG Dongliang

doi:10.37188/CJL.20230048

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Construction of Quantum Dot-modified Ln-ZIF Hybrid Materials and Fluorescence Detection of Tannic Acid

Luminescence Applications and Interdisciplinary Fields | 更新时间：2023-09-28

- Construction of Quantum Dot-modified Ln-ZIF Hybrid Materials and Fluorescence Detection of Tannic Acid
- Chinese Journal of Luminescence Vol. 44, Issue 9, Pages: 1681-1692(2023)
- 作者机构：
  
  上海理工大学材料与化学学院，上海　200093
- 作者简介：
- 基金信息：
  
  国家自然科学基金(21101107;51173107);污染控制与资源化国家重点实验室基金项目(PCRRF19017)
- DOI：10.37188/CJL.20230048
  CLC： TB333
- Published：05 September 2023，
  
  Received：01 March 2023，
  
  Revised：14 March 2023，
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方舟,贾东升,李天铭等.量子点修饰Ln⁃ZIF杂化材料的构筑及其对单宁酸的荧光检测[J].发光学报,2023,44(09):1681-1692.

FANG Zhou,JIA Dongsheng,LI Tianming,et al.Construction of Quantum Dot-modified Ln-ZIF Hybrid Materials and Fluorescence Detection of Tannic Acid[J].Chinese Journal of Luminescence,2023,44(09):1681-1692.
方舟,贾东升,李天铭等.量子点修饰Ln⁃ZIF杂化材料的构筑及其对单宁酸的荧光检测[J].发光学报,2023,44(09):1681-1692. DOI： 10.37188/CJL.20230048.

FANG Zhou,JIA Dongsheng,LI Tianming,et al.Construction of Quantum Dot-modified Ln-ZIF Hybrid Materials and Fluorescence Detection of Tannic Acid[J].Chinese Journal of Luminescence,2023,44(09):1681-1692. DOI： 10.37188/CJL.20230048.

摘要

采用一步水热法制备了一种具有新型褶皱球结构的镧系金属Eu

掺杂的金属有机骨架材料Eu/ZIF⁃67，并进一步通过配位键合的方式将ZnO量子点负载到Eu/ZIF⁃67的表面，形成了一种类沸石咪唑酯骨架的双发射荧光杂化材料Eu/ZIF⁃67@ZnO QDs。通过对材料的结构、形貌以及荧光传感性能表征分析，发现该荧光材料具有ZnO量子点和镧系红光铕离子的双重荧光发射。此外，进一步探究了Eu/ZIF⁃67@ZnO QDs对单宁酸的荧光传感性能。结果表明，单宁酸能够有效猝灭Eu/ZIF⁃67@ZnO QDs在ZnO QDs处的特征荧光发射，检出限为0.029 9 µmol/L。同时，Eu/ZIF⁃67@ZnO QDs对单宁酸的荧光响应具有抗干扰能力，可作为一种经济高效的荧光传感器来特异性识别单宁酸。

Abstract

Lanthanide Eu

-doped metal-organic backbone material Eu/ZIF-67 was prepared by a one-step hydrothermal method with a novel pleated sphere structure. A dual-emission fluorescent hybrid material Eu/ZIF-67@ZnO QDs with a zeolite imidazolium ester backbone was obtained by loading ZnO quantum dots onto the surface of Eu/ZIF-67

via

coordination bonding. The structure， morphology and fluorescence sensing properties of the material were characterized in detail. Furthermore， the fluorescent material was found to display the dual fluorescence emission of ZnO quantum dots and lanthanide red europium ions. The fluorescence sensing performance of Eu/ZIF-67@ZnO QDs to tannic acid was further investigated， and the results indicated that tannic acid can effectively burst the characteristic fluorescence emission of Eu/ZIF-67@ZnO QDs at ZnO QDs with a detection limit of 0.029 9 µmol/L. Meanwhile， Eu/ZIF-67@ZnO QDs have the fluorescence response to tannic acid with anti-interference ability， which can be used as a cost-effective fluorescence sensor to specifically identify tannic acid.

关键词

金属有机骨架量子点双发射探针单宁酸荧光检测

Keywords

metal organic skeletonquantum dotsdual-emission probestannic acidfluorescent detection

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⁰

Construction of Quantum Dot-modified Ln-ZIF Hybrid Materials and Fluorescence Detection of Tannic Acid

DOI：10.37188/CJL.20230048

摘要

Abstract

关键词

Keywords

references