Progress in Preparation and Application of Biomass-based Carbon Quantum Dots

WANG Shi-peng; DONG Ya-hui; ZHAO Hao-ran; LI Yu; CHENG Qian

doi:10.37188/CJL.20220063

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Progress in Preparation and Application of Biomass-based Carbon Quantum Dots

Synthesis and Properties of Materials | 更新时间：2022-10-19

- Progress in Preparation and Application of Biomass-based Carbon Quantum Dots
  增强出版
- Chinese Journal of Luminescence Vol. 43, Issue 6, Pages: 833-850(2022)
- 作者机构：
  
  1.东北林业大学生物质材料科学与技术教育部重点实验室，黑龙江哈尔滨　 150040
  2.东北林业大学理学院，黑龙江哈尔滨　150040
- 作者简介：
- 基金信息：
  
  Fundamental Research Funds for the Central Universities(2572019BB06);Heilongjiang Provincial Natural Science Foundation(HL2019E002)
- DOI：10.37188/CJL.20220063
  CLC：
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王士鹏,董娅慧,赵浩然等.生物质基碳点制备及应用研究进展[J].发光学报,2022,43(06):833-850.

WANG Shi-peng,DONG Ya-hui,ZHAO Hao-ran,et al.Progress in Preparation and Application of Biomass-based Carbon Quantum Dots[J].Chinese Journal of Luminescence,2022,43(06):833-850.
王士鹏,董娅慧,赵浩然等.生物质基碳点制备及应用研究进展[J].发光学报,2022,43(06):833-850. DOI： 10.37188/CJL.20220063.

WANG Shi-peng,DONG Ya-hui,ZHAO Hao-ran,et al.Progress in Preparation and Application of Biomass-based Carbon Quantum Dots[J].Chinese Journal of Luminescence,2022,43(06):833-850. DOI： 10.37188/CJL.20220063.

摘要

碳点（CDs）作为一种新型的碳纳米荧光材料，因具有易制备、光学性能稳定、低毒和良好的生物相容性等优点而备受关注。然而，其荧光性能调控、荧光量子产率（QY）改善、寻求绿色环保和可持续发展的碳源仍是实现其多方面应用的关键。生物质材料在自然界中广泛存在、种类丰富且能够重复再生，在CDs制备过程中可同时控制碳核和表面态的形成，进而实现荧光性能调控和QY改善，作为来源广、廉价易得的碳源引起了科学家的广泛关注。本文从CDs的发光颜色调控出发对近年来生物质基CDs的绿色制备进行综述，分析归纳了不同生物质材料作为碳源及制备方法对生物质基CDs的发光颜色和QY的影响，梳理并总结了生物质基CDs在生物成像、药物递送、传感、防伪、光催化及LED等方面的应用研究进展，同时对生物质基CDs的性能优化、绿色制备方法面临的挑战及未来的发展方向进行了展望。

Abstract

Carbon dots（CDs）， as a novel carbon nanofluorescent material， has attracted much attention due to its advantages of easy preparation， stable optical properties， low toxicity and good biocompatibility. However， the regulation of fluorescence properties， the improvement of fluorescence quantum yield（QY） and the search for green and sustainable carbon source are the key to realize its multifaceted application. Biomass materials have attracted extensive attention of scientists due to being widely existed in nature， rich in variety and capable of repeated regeneration. In the process of CDs preparation， the formation of carbon nuclei and surface states can be controlled simultaneously， which result in regulating the fluorescence performance and improving QY. In this paper， the researches on the green synthesis of biomass derived CDs（B-CDs） based on the regulation of the emitting light colors in recent years are summarized. And the effect on the fluorescence color and QY is analyzed according to the selection of biomass carbon source and synthesis method. Furthermore， the applications of B-CDs in biological imaging， drug delivery， sensing， anti-counterfeiting， photocatalysis and LED are discussed. At the same time， the challenges and future development direction of B-CDs in the aspects of performance optimization and green synthesis method are also prospected.

关键词

生物质基碳点绿色合成光致发光量子效率生物应用

Keywords

biomass derived carbon dotsgreen synthesisphotoluminescencequantum yieldbiomedical applications

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王士鹏（1997-），男，辽宁葫芦岛人，硕士研究生，2020年于沈阳航空航天大学获得学士学位，主要从事碳量子点和纳米纤维素水凝胶等方面的研究。. doi: 10.1016/j.orgel.2021.106255http://dx.doi.org/10.1016/j.orgel.2021.106255

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