Preparation and Performance of Luminescent Solar Concentrator Based on Surface Plasmon Resonance Effect

Xiu-dong CAO; Hui-hong ZHANG; Ye TIAN; Yi ZHANG; Gang-wei GU; Xiao-wei ZHANG

doi:10.37188/CJL.20210387

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Preparation and Performance of Luminescent Solar Concentrator Based on Surface Plasmon Resonance Effect

Device Fabrication and Physics | 更新时间：2022-04-07

- Preparation and Performance of Luminescent Solar Concentrator Based on Surface Plasmon Resonance Effect
  增强出版
- Chinese Journal of Luminescence Vol. 43, Issue 3, Pages: 396-403(2022)
- 作者机构：
  
  1.宁波大学　信息科学与工程学院，浙江　宁波　315211
  2.南京大学　固体微结构国家重点实验室，江苏　南京　210093
- 作者简介：
- 基金信息：
  
  Foundation of China(61974078;61704094);Natural Science Foundation of Zhejiang Province(LY21F040002);Fundamental Research Funds for the Provincial Universities of Zhejiang(SJLY2021012)
- DOI：10.37188/CJL.20210387
  CLC：
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Xiu-dong CAO, Hui-hong ZHANG, Ye TIAN, et al. Preparation and Performance of Luminescent Solar Concentrator Based on Surface Plasmon Resonance Effect. [J]. Chinese Journal of Luminescence 43(3):396-403(2022)
DOI：

Xiu-dong CAO, Hui-hong ZHANG, Ye TIAN, et al. Preparation and Performance of Luminescent Solar Concentrator Based on Surface Plasmon Resonance Effect. [J]. Chinese Journal of Luminescence 43(3):396-403(2022) DOI： 10.37188/CJL.20210387.

摘要

金属纳米颗粒的表面等离子体共振效应能够对特定波长入射光的吸收或者散射增强，正因为其独特的光学性质，金属纳米颗粒被尝试应用于荧光太阳集光器。本文利用全无机钙钛矿CsPbBr,3,量子点、Au纳米颗粒和硫醇-烯聚合物制备荧光太阳集光器。研究发现，掺杂适量Au纳米颗粒可以通过表面等离子体共振效应提高全无机钙钛矿CsPbBr,3,量子点荧光太阳集光器的外量子效率。当Au纳米颗粒的掺杂浓度为2.0×10,-6,时，荧光太阳集光器的外量子效率为12.3%，相比未掺杂Au纳米颗粒的荧光太阳集光器的外量子效率提升了78.2%。进一步提高Au纳米颗粒的掺杂浓度，荧光太阳集光器的外量子效率下降。荧光发射谱和荧光寿命谱测试结果显示，当Au纳米颗粒的掺杂浓度超过2.0×10,-6,时，过高的Au纳米颗粒掺杂浓度导致CsPbBr,3,量子点与Au纳米颗粒之间发生非辐射能量转移，荧光太阳集光器荧光量子产率(,η,PL,LSC,)下降导致了外量子效率下降。

Abstract

The surface plasmon resonance effect of metal nanoparticles can enhance the absorption and scattering of incident light at a certain wavelength. Because of this unique optical property, the metal nanoparticles are developed for the applications of luminescent solar concentrators. In this paper, the Au nanoparticles with different concentrations are introduced to the luminescent solar concentrators based on the all-inorganic perovskite CsPbBr,3, quantum dots and the thiol-ene polymer. The results show that the Au nanoparticles with suitable concentration can improve the external quantum efficiency of the luminescent solar concentrators by the surface plasmon resonance effect. When the doping concentration of Au nanoparticles is 2.0×10,-6, the external quantum efficiency of the luminescent solar concentrator is 12.3%, which is enhanced by 78.2% compared with that of Au-free luminescent solar concentrator. With the further increase of Au nanoparticle doping concentration above 2.0×10,-6, the external quantum efficiency of the luminescent solar concentrators decreases. According to the photoluminescence emission spectra and the time-resolved photoluminescence emission curves, excessive Au nanoparticle doping concentration leads to the non-radiative energy transfer process between the CsPbBr,3, quantum dots and Au nanoparticles. The decreasing fluorescence quantum yield(,η,PL,LSC,) gives rises to decreasing external quantum efficiency of the luminescent solar concentrator.

关键词

钙钛矿量子点Au纳米颗粒表面等离子体共振效应外量子效率非辐射能量转移

Keywords

perovskite quantum dotAu nanoparticlesurface plasmon resonance effectexternal quantum efficiencynon-radiative energy transfer

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