Effect of Ta<sub>2</sub>O<sub>5</sub> on Optical Properties of Tellurium Bismuthate Glass

Jia-hang LI; Jia YU; Mei-feng HU; Hui-dan ZENG; Xiao-feng LIU

doi:10.37188/CJL.20210382

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Effect of Ta₂O₅ on Optical Properties of Tellurium Bismuthate Glass

Synthesis and Properties of Materials | 更新时间：2022-04-07

- Effect of Ta₂O₅ on Optical Properties of Tellurium Bismuthate Glass
  增强出版
- Chinese Journal of Luminescence Vol. 43, Issue 3, Pages: 371-380(2022)
- 作者机构：
  
  1.华东理工大学　材料科学与工程学院，上海　200237
  2.浙江大学　材料科学与工程学院，浙江　杭州　310027
- 作者简介：
- 基金信息：
  
  National Natural Science Foundation of China(51872092;52072122)
- DOI：10.37188/CJL.20210382
  CLC： TQ171.733
- Published：2022-03，
  
  Received：07 December 2021，
  
  Revised：24 December 2021，
- 稿件说明：
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JIA-HANG LI, JIA YU, MEI-FENG HU, et al. Effect of Ta₂O₅ on Optical Properties of Tellurium Bismuthate Glass. [J]. Chinese journal of luminescence, 2022, 43(3): 371-380.
DOI：

JIA-HANG LI, JIA YU, MEI-FENG HU, et al. Effect of Ta₂O₅ on Optical Properties of Tellurium Bismuthate Glass. [J]. Chinese journal of luminescence, 2022, 43(3): 371-380. DOI： 10.37188/CJL.20210382.

摘要

通过高温熔融法制备了一系列(90-

)TeO

-10Bi

(

=0%

8%)TBT玻璃样品。拉曼光谱和X射线光电子能谱测试结果显示，随着Ta

的加入，玻璃网络中的［TeO

］与［TeO

3+1

］向［TeO

］转变，玻璃网络结构更加致密。这解释了差示扫描量热法测试中TBT玻璃的玻璃化转变温度

随Ta

的含量增加而增加的变化原因。当Ta

从0升高到8%，吸收光谱以及光学带隙方程计算表明，玻璃样品的光学带隙和乌尔巴赫能(Urbach)不断降低。使用

扫描方法测试了各个TeO

-Bi

-Ta

玻璃样品的三阶非线性光学特性，结果表明，TBT玻璃的三阶非线性与Ta

的加入量呈正相关。当Ta

的加入量为8%时，其三阶非线性极化率为3.30×10

-20

·V

-2

(2.36×10

-12

esu)，这表明该组成的碲铋酸盐玻璃在非线性光学领域具备潜在的应用价值。

Abstract

By using differential scanning calorimetry(DSC) method

this research indicates glass transition temperture(

) of a series of (90-

)TeO

-10Bi

(

=0%

8%)(TBT) glass is increased with more Ta

added. The phenomenon of increasing

is mainly contributed to transformation of [TeO

] and [TeO

3+1

] to [TeO

] units. And the structure changes result in highly dense glass network structure which is supported by Raman spectroscopy and XPS charactreizations. Based on results of absorption spectrum and optical band gap equation calculation

when Ta

increases from 0 to 8%

the optical band gap and Urbach energy of such glass samples show decresing trends. The third-order nonlinear optical properties of TBT glass demonstrate positive correlation with concentration of Ta

through

Z-

scan measurement. The TBT glass with 8% Ta

has 3.30×10

-20

·V

-2

(2.36×10

-12

esu) of third-order nonlinear susceptibility. Thus

the outstanding properties of TBT glasses pave a way of nonlinear optical applications.

关键词

碲酸盐玻璃氧化钽非线性光学

Keywords

tellurite glasstantalum oxidenonlinear optics

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Related Author

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Related Institution

School of Materials Science and Engineering， Zhejiang University

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⁰

Effect of Ta2O5 on Optical Properties of Tellurium Bismuthate Glass

DOI：10.37188/CJL.20210382

摘要

Abstract

关键词

Keywords

references

Effect of Ta₂O₅ on Optical Properties of Tellurium Bismuthate Glass