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Research Progresses of Photoluminescence and Application for Emerging Zero-dimensional Metal Halides Luminescence Materials
增强出版- Chinese Journal of Luminescence Vol. 42, Issue 6, Pages: 733-754(2021)
- 作者机构：
1.华南理工大学材料科学与工程学院 发光材料与器件国家重点实验室，广东省光纤激光材料与应用技术重点实验室, 广东 广州 510640
2.华南理工大学 物理与光电学院, 广东 广州 510640
- 作者简介：
- 基金信息：National Natural Science Foundation of China(51961145101;51972118);Guangzhou Science and Technology Project(202007020005);Local Innovative and Research Teams Project of Guangdong Pearl River Talents Program(2017BT01X137)
DOI：10.37188/CJL.20210088
CLC： O482.31Published：01 June 2021，
Received：12 March 2021，
Revised：29 March 2021，
扫 描 看 全 文
Bin-bin SU, Zhi-guo XIA. Research Progresses of Photoluminescence and Application for Emerging Zero-dimensional Metal Halides Luminescence Materials. [J]. Chinese Journal of Luminescence 42(6):733-754(2021)
Bin-bin SU, Zhi-guo XIA. Research Progresses of Photoluminescence and Application for Emerging Zero-dimensional Metal Halides Luminescence Materials. [J]. Chinese Journal of Luminescence 42(6):733-754(2021) DOI： 10.37188/CJL.20210088.
摘要
零维(0D)金属卤化物是一类新兴的发光材料体系，它们具有独特的“主-客”体结构，即独立的阴离子金属卤化物多面体客体规则有序地分布在有机阳离子或碱金属阳离子形成的主体框架中。这种具有相对较“软”晶格的0D金属卤化物材料的发光主要源于自陷激子(Self-trapped excitons
STEs)复合，其通常呈现出宽带发射，且具有大的斯托克斯位移。通过筛选不同的及多样化构型的金属卤化物多面体，将其与合适的有机阳离子或者Cs
+
等组合，可形成多种新型结构的0D金属卤化物，并实现丰富的STEs发光特性，其可调节的荧光发射不仅可以覆盖整个可见光区，还可实现单相白光或近红外发光，成为光致发光材料研究领域的一个热点和重点。基于此，本文结合本课题组在该领域的研究工作基础，首先讨论了0D金属卤化物的光致发光机理;其次，介绍了具有不同多面体构型的0D金属卤化物材料的发光特性及应用;最后，总结了0D金属卤化物目前亟待解决的关键科学问题，并对0D金属卤化物的未来发展方向进行了展望。
Abstract
Zero-dimensional(0D) metal halides belong to a new kind of luminescent materials
and they have the unique "host-guest" structure
in which the isolated anionic metal halide polyhedrons are regularly distributed in the main body of organic cations or alkali metal ions. Generally
0D metal halides with relatively "soft" lattice usually present broad band emission with large Stokes shift
and their luminescence mechanism is mainly derived from self-trapped excitons(STEs) recombination. By screening different metal halide polyhedrons with diversified configurations
one can combine them with appropriate organic cations or alkali metal ions to form new 0D metal halides with different structure types. The obtained 0D metal halides show rich STEs luminescence properties
and their tunable fluorescence emission can be available to cover the entire visible light region. Moreover
it can also realize single-phase white light emission or near infrared emission
making them become a hot spot in the field of photoluminescence materials. Based on our work and others in this field
the photoluminescence mechanisms of 0D metal halides are firstly discussed in this review. Secondly
the luminescence properties and applications of 0D metal halide materials with different polyhedron configurations are introduced. Finally
the key scientific problems of 0D metal halides during the development are summarized
and the future research direction is briefly proposed.
关键词
金属卤化物光致发光LED应用
Keywords
metal halidesphotoluminescenceLED application
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