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1. 南京大学, 物理系,江苏 南京,210093
2. 华侨大学, 信息科学与工程学院,福建 泉州,362021
3. 中国科学院, 半导体研究所 北京,100083
收稿:2007-09-21,
修回:2008-1-4,
纸质出版:2008-11-20
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申继伟, 郭亨群, 吕蓬, 徐骏, 陈坤基, 王启明. Si/SiN<sub>x</sub>超晶格材料的非线性光学特性[J]. 发光学报, 2008,29(6): 1045-1049
SHEN Ji-wei, GUO Heng-qun, LU Peng, XU Jun, CHEN Kun-ji, WANG Qi-ming. Nonlinear Optical Properties of Si/SiN<sub>x</sub> Superlattice[J]. Chinese Journal of Luminescence, 2008,29(6): 1045-1049
采用射频磁控反应溅射技术与热退火处理制备了Si/SiN
x
超晶格材料.利用吸收光谱和X射线衍射对材料进行表征.通过皮秒脉冲激光单光束Z-扫描技术研究了该材料在非共振吸收区的三阶非线性光学特性
实验结果表明
样品的非线性折射率为负值
非线性吸收属于双光子吸收.由实验数据得到材料的三阶非线性极化率实部和虚部分别为1.27×10
-7
1.1×10
-8
esu
该值比体硅材料的三阶非线性极化率值大个数量级.对材料光学非线性产生的机理进行了探讨
认为材料的非线性极化率的增加来源于材料量子限制效应的增强.
In order to study preparation process recipes and nonlinear optical properties of Si/SiN
x
superla-ttice
Si/SiN
x
superlattice has been fabricated by RF magnetron sputtering technique and thermal annealing.The superlattice has been characterized by absorption measurement
and X-ray diffraction.Nonlinear optical properties of Si/SiN
x
superlattice was probed by a Z-scan technique at λ=1064 nm.The experimental results show that the nonlinear refractive index of the sample is a negative value and the nonlinear absorption is two-photon absorption.The real and imaginary parts of χ
(3)
have been found to be 1.27×10
-7
(esu)and 1.51×10
-8
(esu)according to the experimental data of Z-scan curve.The value of Si/SiN
x
superlattice is larger 5 scales than that of bulk silicon.The nonlinear mechanism of the material was discussed.The enhancement of non-linear refractive index is mainly attributed to intensive quantum confinement.The results indicate that such Si/SiN
x
superlattice material could be applied to the optoelectronics and microelectronics industry since it is compatible with Si technology.
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