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1. 中国科学院激发态物理开放研究实验室, 中国科学院长春光学精密机械与物理研究所, 吉林, 长春, 130021
2. 东北师范大学化学系, 吉林, 长春, 130024
收稿日期:2001-08-17,
修回日期:2001-09-15,
纸质出版日期:2001-11-30
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刘俊业, 刘春旭, 张立功, 黄宗浩, 关宏宇, 张家骅, 许武. 含纳米随机微腔MEH-PPV/玻璃光波导激光[J]. 发光学报, 2001,22(4): 405-408
LIU Jun-ye, LIU Chun-xu, ZHANG Li-gong, HUANG Zong-hao, GUAN Hong-yu, ZHANG Jia-hua, XU Wu. MEH-PPV/Glass Waveguide Laser with Random Nanoparticles Microcavities[J]. Chinese Journal of Luminescence, 2001,22(4): 405-408
刘俊业, 刘春旭, 张立功, 黄宗浩, 关宏宇, 张家骅, 许武. 含纳米随机微腔MEH-PPV/玻璃光波导激光[J]. 发光学报, 2001,22(4): 405-408 DOI:
LIU Jun-ye, LIU Chun-xu, ZHANG Li-gong, HUANG Zong-hao, GUAN Hong-yu, ZHANG Jia-hua, XU Wu. MEH-PPV/Glass Waveguide Laser with Random Nanoparticles Microcavities[J]. Chinese Journal of Luminescence, 2001,22(4): 405-408 DOI:
用浸涂法制备了MEH-PPV/TiO
2
重量比分别为1:0
1:1
1:2和1:3四种不同纳米微晶薄膜.与已报道的亚微米散射体不同
本实验采用粒径约为20nm的TiO
2
纳米微晶作为多重散射体.可以不必考虑光在散射体上的出、入射方向和内部传播情况.飞秒激光器经OPA调谐产生脉宽为130fs的超短脉冲
激发波长为544nm
重复频率为1kHz
激发功率为3μJ/pulse.研究了不同激发强度下
光谱的增益窄化
激射强度和与激发光条长度的关系.这种激光发射的本质还是放大自发辐射(ASE)为主.分析了在平均自由程
l
=5.4×10
5
nm下光的输运和光局域对这种随机激光产生的影响.
The four kinds of films MEH-PPV(1mg)/ml
[MEH-PPV(1mg)+TiO
2
(1mg)]/ml
[MEH-PPV(1mg)+TiO
2
(2mg)]/ml and [MEH-PPV( 1mg)+TiO
2
(3mg)]/ml were made by dip coating method.The diameters of the scatters TiO
2
are of submicrometer in all reports published before in films or solutions.Random lasing with the scatters of 20nm has been reported in this letter.The femtosecond laser through OPA hamornics produce 130fs pulse duration
544nm exciting wavelength
1kHz repeat ratio
and 3~μJ/pulse pump power.The spectrum line narrowed dramatically almost in two orders of magnitude
smaller than the spectrum lines excited by Xenon lampe.The outputs on the end of the film were exponen-tially increased with lengthening the excitation stripe of laser beam.It is shown that the amplified sponta-neous emission(ASE) is the dominant mechanism.The effects of Anderson location of light on random las-ing with the mean free path
l
=5.4×10
5
nm were discussed.
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