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1. 北京师范大学物理系, 北京 10087
2. 广州师范学院物理系, 广东广州 510405
收稿日期:2000-06-29,
修回日期:2000-11-10,
纸质出版日期:2001-05-30
移动端阅览
刘翠红, 郭康贤, 陈传誉, 马本堃. 量子盘中的三阶非线性光学极化率[J]. 发光学报, 2001,22(2): 135-138
LIU Cui-hong, GUO Kang-xian, CHEN Chuan-yu, MA Ben-kun. Third-order Nonlinear Optical Susceptibility in Quantum Disks[J]. Chinese Journal of Luminescence, 2001,22(2): 135-138
利用密度矩阵方法讨论了量子盘中的三阶非线性光学极化率
导出了近共振条件下的三次谐波的解析表达式
并以GaAs量子盘为例进行了具体的计算。结果表明
GaAs量子盘中的三阶非线性光学极化率要比GaAs量子阱的大几十倍。而且
选取适当的参量
可在吸收系数相对较小的情况下获得较大的折射率。
In recent years
the subject of optical nonlinearity in semiconductor quantum confined structures such as quantum wires and quantum dots has attracted a considerable attention because of their relevance for studying practical applications and as a probe for the electronic structure of media.It has been shown that the low-dimensional quantum systems present very large nonlinear optical susceptibilities.Theoretically
most of the studies on quantum dots are focused on spherical quantum dots for simplicity.The shape of quantum dot depends on growth conditions.In fact
quantum dots are better described as thin disk or cylinder.In the present work third-order nonlinear optical susceptibilities in disk-shaped quantum dots due to resonant intersubband transition are analyzed by a compact density matrix approach.It has rarely been discussed in literatures.Firstly
we consider an electron moving in a quantum disk whose radius
R
is very large compared to its thickness d.For simplicity
we assume that the isotropic effective mass approximation is valid within the disk and that the inner potential is null while the outer confining potential is approximately infinite.Using the adiabatic approximation we solve the three dimensional Schr-dinger equation and obtain the analytical expressions of wave functions and energy levels in cylindrical coordinates.Secondly
we consider the system is excited by an electromagnetic field with frequency ω. The electromagnetic field is incident with a polarization vector normal to the disk.We treat
H
'=ez
E
(
t
) as a perturbation term.By using the compact density matrix method
we derive a general formula for third order nonlinear optical susceptibilites employing a four-level model in quantum disk.Finally
numerical results are illustrated for a typical GaAs quantum disk.We calculate the third-order nonlinear optical susceptibilities as a function of the disk thickness.It is shown that the third order nonlinear optical susceptibilities in quantum disk are 10~100 times larger than that in quantum well for various disk thickness.Furthermore
if we choose an optimized thickness of quantum disk
we could obtain a quite large refractive index with a comparatively small absorption coefficient.Therefore
we suggest that the quantum dots would be an excellent system in the field of optical communications and optical switching.
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