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1. 中国科学院长春光学精密机械与物理研究所,吉林 长春,130021
2. 中国科学院激发态物理开放研究实验室,吉林 长春,130021
收稿日期:2000-06-20,
修回日期:2000-08-25,
纸质出版日期:2000-11-30
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范希武, 于广友, 张吉英, 杨宝均, 申德振. ZnCdSe/ZnSe非对称双量子阱中的光学特性研究[J]. 发光学报, 2000,21(4): 293-298
FAN X W, YU Guang-you, ZHANG Ji-ying, YANG Bao-jun, SHEN De-zhen. Optical Characteristics of ZnCdSe/ZnSe Asymmetric Double Quantum Wells[J]. Chinese Journal of Luminescence, 2000,21(4): 293-298
用LP-MOCVD技术在GaAs衬底上外延生长了ZnCdSe/ZnSe非对称双量子阱(ADQW)结构。通过ps时间分辨光谱、吸收光谱、发射光谱等的研究得到了如下的结果:在弱激发下
观测到ADQW结构中的激子隧穿现象;在强激发下
在ADQW结构中发现了一个内建电场
它将影响激子隧穿;首次观测到由激子隧穿引起的在一定温度范围内宽阱的发光强度随温度上升而增加的现象;首次观测到该ADQW结构中来自宽阱的光泵受激发射。
The ZnCdSe/ZnSe asymmetric double quantum wells(ADQW)samples studied were grown on(100)Si-doped GaAs substrates by low pressure(LP)MOCVD. The sample structure consists of a 1μm ZnSe buffer layer followed by ten periodes of Zn
0.72
Cd
0.28
Se/ZnSe ADQW and then a 60nm ZnSe cap layer. Each period of ZnCdSe/ZnSe ADQW includes one narrow ZnCdSe quantum well
one thin ZnSe barrier and one wide ZnCdSe quantum well. Each period of the ADQW was separated by a 40nm ZnSe barrier. Exciton tunneling has been studied in the ZnCdSe/ZnSe ADQW. There are two emission peaks of the time-resolved spectra of the ADQW corresponding to
n
=1 heavy hole recombination from the wide well (WW) and narrow well (NW)
respectively. It is obvious that the
n
=1 heavy hole excitonic emission from the WW dominates the spectra
and the
n
=1 heavy hole excitonic emission from the NW decreases and disappears gradually with increasing the delay time. Considering the exciton tunneling in the ADQW
this phenomenon can be explained. Under stronger excitation
the tunneling of free electron and free hole are also observed in the ADQW. Due to different tunneling time of free electron and free hole
space charge effect was observed in the ADQW
which leaded to the foundation of the internal electric field. The excitation intensity dependence of the luminescence intensity in the WW and NW as shown in fig.5 can be explained by foundation of the internal electric field. The spontaneous and stimulated emission have been studied in the ZnCdSe/ZnSe ADQW. For spontaneous emission of the ADQW
the exciton recombination both in the NW and WW is influenced by two factors
the exciton tunneling and the thermal dissociation processes. For the NW
the two factors have the same influence on the emission intensity
but for the WW
the influence on the emission intensity of two factors are contrary. The change of the emission intensity in the WW is determined by the stronger one. For stimulated emission of the ADQW
owing to the difference of the energy levels between the WW and the NW
the carriers tunnel from the NW to the WW
which can influence the emission effectively.The carrier tunneling is conductive to lasing from the WW.
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