Monte-Carlo Ray-tracing Simulations of Perovskite Quantum Dots-based Luminescent Solar Concentrators

SHU Jun-peng; WANG Peng-jun; ZHANG Xiao-wei; XIE Kai-he; ZHANG Hui-hong; CHEN Ruo-wang

doi:10.3788/fgxb20194004.0484

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Monte-Carlo Ray-tracing Simulations of Perovskite Quantum Dots-based Luminescent Solar Concentrators

Device Fabrication and Physics | 更新时间：2020-08-12

- Monte-Carlo Ray-tracing Simulations of Perovskite Quantum Dots-based Luminescent Solar Concentrators
- Chinese Journal of Luminescence Vol. 40, Issue 4, Pages: 484-490(2019)
- 作者机构：
  
  宁波大学信息科学与工程学院,浙江宁波,315211
- 作者简介：
- 基金信息：
  
  Supported by National Natural Science Foundation of China(61704094,61474068);Research Foundation of Education Bureau of Zhejiang Province(Y201737316);Sponsored by K. C. Wong Magna Fund in Ningbo University
- DOI：10.3788/fgxb20194004.0484
  CLC： O482.31
- Received：25 July 2018，
  
  Revised：10 September 2018，
  
  Published Online：21 September 2018，
  
  Published：05 April 2019
- 稿件说明：
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束俊鹏, 汪鹏君, 张晓伟等. 基于钙钛矿量子点荧光太阳集光器的蒙特卡洛光子追踪模拟[J]. 发光学报, 2019,40(4): 484-490

SHU Jun-peng, WANG Peng-jun, ZHANG Xiao-wei etc. Monte-Carlo Ray-tracing Simulations of Perovskite Quantum Dots-based Luminescent Solar Concentrators[J]. Chinese Journal of Luminescence, 2019,40(4): 484-490
束俊鹏, 汪鹏君, 张晓伟等. 基于钙钛矿量子点荧光太阳集光器的蒙特卡洛光子追踪模拟[J]. 发光学报, 2019,40(4): 484-490 DOI： 10.3788/fgxb20194004.0484.

SHU Jun-peng, WANG Peng-jun, ZHANG Xiao-wei etc. Monte-Carlo Ray-tracing Simulations of Perovskite Quantum Dots-based Luminescent Solar Concentrators[J]. Chinese Journal of Luminescence, 2019,40(4): 484-490 DOI： 10.3788/fgxb20194004.0484.

摘要

传统光聚集器热效应明显、结构复杂、成本昂贵。作为替代，荧光太阳集光器具有许多显著优势并能够有效降低太阳能电池的发电成本，因此受到广泛关注。本文通过传统热注入法合成了全无机钙钛矿CsPbBr

量子点，并在此基础上设计了基于CsPbBr

量子点的荧光太阳集光原型器件。通过TEM测试和必要的光学表征，证实本文合成的CsPbBr

量子点具有典型的立方体结构、76.8%的荧光量子产率、512 nm的发光中心波长和22 nm的中心波长半高宽。此外，结合蒙特卡洛智能优化算法，建立了基于CsPbBr

量子点的荧光太阳集光器的理论计算模型，确定了全无机钙钛矿量子点最优掺杂浓度和最佳平均波长集光效率。仿真结果表明，在量子点掺杂浓度为2.110

-5

mol/L时，最优的集光效率达到5.4%。本文提出的蒙特卡洛光子追踪模拟过程将为未来荧光太阳集光器参数设计提供科学的计算方法。

Abstract

The inevitable thermal effects

complex device structure and high manufacturing cost severely hinder the development of the conventional solar concentrators. As a type of novel solar concentrators

luminescent solar concentrator shows numerous potentials to significantly reduce the cost of solar cells and attracts much attentions. Here

the all-inorganic perovskite CsPbBr

quantum dots are synthesized

via

a hot-injection approach and then the CsPbBr

-based luminescent solar concentrators are designed and fabricated. According to TEM characterization and spectroscopic measurements

the CsPbBr

quantum dots exhibit the typical cubic structure

the quantum yield of up to 76.8%

and the PL emission at 512 nm with the FWHM of 22 nm. Further

the optimal quantum dots doping concentration and the average optical collecting efficiency are confirmed by the calculation based on Monte Carlo intelligent optimization algorithm. The optimal average collecting efficiency is 5.4% when CsPbBr

quantum dots doping concentration is fixed at 2.110

-5

mol/L. We anticipate this numerical simulation process based on Monte Carlo intelligent optimization algorithm will shed light on the future research for determining the characteristic parameter of luminescent solar concentrators.

关键词

Keywords

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