Emission Characteristics of Crown-like ZnO Nanocrystals Induced by Three-photon Absorption and Second Harmonic Generation Effect

WANG Ma-hua; ZHU Guang-ping; JU Yong-feng; FU Li-hui; FU Cheng-fang; ZHAO Zheng-ming; JI R

doi:10.3788/fgxb20153606.0617

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Emission Characteristics of Crown-like ZnO Nanocrystals Induced by Three-photon Absorption and Second Harmonic Generation Effect

更新时间：2020-08-12

- Emission Characteristics of Crown-like ZnO Nanocrystals Induced by Three-photon Absorption and Second Harmonic Generation Effect
- Chinese Journal of Luminescence Vol. 36, Issue 6, Pages: 617-622(2015)
- 作者机构：
  
  1. 淮阴工学院电子与电气工程学院,江苏淮安,223003
  2. 淮北师范大学物理与电子信息学院,安徽淮北,235000
- 作者简介：
- 基金信息：
- DOI：10.3788/fgxb20153606.0617
  CLC： O432.31;O738
- Received：03 April 2015，
  
  Revised：22 April 2015，
  
  Published：03 June 2015
- 稿件说明：
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王马华, 朱光平, 居勇峰等. 纳米氧化锌中三光子吸收与倍频效应致光辐射特性[J]. 发光学报, 2015,36(6): 617-622

WANG Ma-hua, ZHU Guang-ping, JU Yong-feng etc. Emission Characteristics of Crown-like ZnO Nanocrystals Induced by Three-photon Absorption and Second Harmonic Generation Effect[J]. Chinese Journal of Luminescence, 2015,36(6): 617-622
王马华, 朱光平, 居勇峰等. 纳米氧化锌中三光子吸收与倍频效应致光辐射特性[J]. 发光学报, 2015,36(6): 617-622 DOI： 10.3788/fgxb20153606.0617.

WANG Ma-hua, ZHU Guang-ping, JU Yong-feng etc. Emission Characteristics of Crown-like ZnO Nanocrystals Induced by Three-photon Absorption and Second Harmonic Generation Effect[J]. Chinese Journal of Luminescence, 2015,36(6): 617-622 DOI： 10.3788/fgxb20153606.0617.

摘要

为研究强光激励下纳米氧化锌发光机制

以气相传输法制备的冠状样品为对象

室温下以1 100 nm与1 150 nm脉冲激光以及350 nm氙灯对其进行激励

观测光致发光谱。根据光强关系和强场与物质作用的三阶微扰理论

认为 1 100

1 150 nm激光激励下的样品的紫外与可见光波段的辐射机理分别归因于样品中三光子吸收和二次谐波效应。同时

基于激子非弹性碰撞复合机制

对紫外辐射的红移现象进行了分析。

Abstract

For the sake of investigating the photoluminescence (PL) characteristics and the mechanims from zinc oxide nanocrystals

the crown-like nanostructural samples prepared by vapor phase transport method were excited by laser pulse and Xe-lamp. Under 1 100 nm and 1 150 nm excitation

the ultroviolet emission at 388 nm and visible emission at 575 nm were observed. Based on the third disturbation theory of the interaction between intensive light field and matter and the relationship between the emission intensity and excitation power

it is confirmed that the emission performances under 1 100 nm and 1 150 nm excitation should be attributed to the three-photon absorption process and the second harmonic generation effects. Moreover

the redshift phenomena of the ultroviolet emission was analyzed based on the exciton-exciton inelastic collision recombination process.

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references

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