Influence of Silver Nanocrystallites on The Upconversion Properties in Tm/Yb Co-doped Tellurite Glasses

ZHANG Wen-jun; LIN Jian; SUN Guang-yao; JIA Yu-jie; QIAN Shuai; REN Jun-jiang; RONG Liang

doi:10.3788/fgxb20133405.0559

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Influence of Silver Nanocrystallites on The Upconversion Properties in Tm/Yb Co-doped Tellurite Glasses

更新时间：2020-08-12

- Influence of Silver Nanocrystallites on The Upconversion Properties in Tm/Yb Co-doped Tellurite Glasses
- Chinese Journal of Luminescence Vol. 34, Issue 5, Pages: 559-564(2013)
- 作者机构：
  
  1. 同济大学材料科学与工程学院上海,201804
  2. 同济大学先进土木工程材料教育部重点实验室上海,200092
  3. 中国电子科技集团公司第二十三研究所上海,200437
- 作者简介：
- 基金信息：
- DOI：10.3788/fgxb20133405.0559
  CLC： O482.31
- Received：24 January 2013，
  
  Revised：16 March 2013，
  
  Published：10 May 2013
- 稿件说明：
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张文俊, 林健, 孙光耀, 贾玉洁, 钱帅, 任军江, 戎亮. Ag纳米晶对Tm/Yb共掺碲酸盐玻璃上转换发光性能的影响[J]. 发光学报, 2013,34(5): 559-564

ZHANG Wen-jun, LIN Jian, SUN Guang-yao, JIA Yu-jie, QIAN Shuai, REN Jun-jiang, RONG Liang. Influence of Silver Nanocrystallites on The Upconversion Properties in Tm/Yb Co-doped Tellurite Glasses[J]. Chinese Journal of Luminescence, 2013,34(5): 559-564
张文俊, 林健, 孙光耀, 贾玉洁, 钱帅, 任军江, 戎亮. Ag纳米晶对Tm/Yb共掺碲酸盐玻璃上转换发光性能的影响[J]. 发光学报, 2013,34(5): 559-564 DOI： 10.3788/fgxb20133405.0559.

ZHANG Wen-jun, LIN Jian, SUN Guang-yao, JIA Yu-jie, QIAN Shuai, REN Jun-jiang, RONG Liang. Influence of Silver Nanocrystallites on The Upconversion Properties in Tm/Yb Co-doped Tellurite Glasses[J]. Chinese Journal of Luminescence, 2013,34(5): 559-564 DOI： 10.3788/fgxb20133405.0559.

摘要

在稀土离子掺杂碲酸盐玻璃中引入Ag纳米晶

通过等离子共振(SPR)可使荧光发射得到增强

上转换发光效率得到明显提升。研究了Ag纳米晶对Tm

/Yb

共掺碲酸盐玻璃上转换发光的影响

分析了上转换发光机理。结果发现

经过(330℃

30 min)热处理后

玻璃中析出了Ag纳米颗粒

尺寸为5~8 nm。Ag纳米晶的引入可使玻璃上转换蓝、红光由三光子吸收转变为双光子吸收。由于局域场表面等离子体共振增强以及Ag与Tm

之间的能量转移

使得含Ag纳米晶玻璃的荧光强度比不含Ag纳米晶的玻璃提高了约5倍。

Abstract

By introducing Ag nanocrystallites into rare earth ions doped tellurite glass

the fluorescence intensity were enhanced through surface plasmon resonance (SPR)

and the up-conversion luminous efficiency were improved obviously. The influence of Ag nanocrystallites on Tm

/Yb

co-doped tellurate glass was studied

and the up-conversion luminescence mechanism was also discussed. The results show that Ag nanocrystallites with the size from 5 to 8 nm were gained by heat treatment under 330℃ for 30 min. After introducing Ag nanocrystallites

the three-photon absorption of blue-red transition in glass turn to two-photon absorption. Because of the enhanced local field surface plasmon resonance and the energy transfer between Ag and Tm

the fluorescence intensity of Ag-contained glass is 5 times more than glass without Ag nanocrystallites.

关键词

Keywords

references

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